Physics & Astronomy: Faculty Publications

Investigation of Third-Order Optical Nonlinearity in KBe2BO3F2 by Z-Scan

Document Type

Article

Publication Date

8-2012

Publication Title

Applied Physics B

DOI

10.1007/s00340-012-4985-x

Abstract

The third-order optical nonlinearity of deep-ultraviolet (DUV) nonlinear optical (NLO) crystal KBe2BO3F2 (KBBF) was investigated using single-beam Z-scan technique for the first time. The Z-scans were performed on a c-cut KBBF crystal and a KBBF prism-coupling device (PCD) with picosecond pulses at 355 nm. No two-photon absorption was observed in the experiment. The measured nonlinear refraction index n 2 showed positive signs, indicating self-focusing Kerr effects. The n 2 values were estimated to be (1.75±0.35)×10−15 cm2/W with the c-cut sample and (1.85±0.37)×10−15 cm2/W with the PCD, corresponding to the third-order nonlinear optical susceptibilitiesχ(3)effof (0.99±0.20)×10−13 esu and (0.94±0.19)×10−13 esu, respectively. The results are expected to promote the investigation of frequency conversion processes with ultra-short laser in KBBF crystal.

Copyright

This work is archived and distributed under the repository's Standard Copyright and Reuse License (opens in new tab). End users may copy, store, and distribute this work without restriction. For all other uses, permission must be obtained from the copyright owners or their authorized agents.

Share

COinS